Some day soon I am going to do a build thread on this whole idea of turning a FJ40 into a daily driver that is just as comfy on the highway as it is on the trail. This is what I set out to to for my wife when we bought ours two years ago. It is a 75.
I have not done the thread yet because I am embarrassed by my naive assumptions at the onset of this undertaking. Anyway, I am running a 2F with ceramic tuned headers and HEI ignition, so maybe a very mild increase over stock power. We converted to an H55F, 35x12.5 tires, kept the stock gears and did an SOA with spring flips, hoping to gain some perception of increase stability with the longer wheel base (justification but it sure sounds good).
We converted to mini-truck power steering at first, and I hated it. Seeking the ultimate steering, recently went to a saginaw conversion with full PSC ram assist components.
This is stupid expensive and well beyond where I thought I would be at this point in the build. But.....the rig steers with one finger (but I use both hands) and the steering is very tight and smooth on the road. Stop to stop without the slightest resistance parked on dry pavement. The engine purrs smoothly at 65 mph. On steep hills, that's what fourth is for as mentioned earlier in this thread. I had thought about going the the later 3.70 gears but I am sure glad I avoided that mistake, since the rig is a bit under-geared with this combination currently.
Add in a tilt steering column and smaller wheel, and many other creature comforts to be covered later and, well, she's a pretty decent DD for a fast tractor!

I am still in pursuit of the ultimate on / off road FJ40 combination. The bottom line is that this goal is a deep rabbit hole indeed.
The punch line here is that I would never want to drive it over 65 on the highway. It does so without the slightest complaint and up the hills as well. But just can't argue with geometry and gravity now can you?

But, I never planned on needing or wanting to drive over 65 so this part is not frustrating at all. So, you can make one a lot smoother, quieter and easier to drive but I share the opinions of others here who would question excessive speed as part of that goal.

Rob