Needle scalers are pretty sweet but I wouldn't want to do my whole frame with one, especially if a lot of it isn't thick rust (and especially if you don't have a compressor that can keep up with high CFM air tools-- big difference between airing up tires or running an impact and running air tools like this). I'd get a wire wheel for an angle grinder and maybe one of the cup styles. Any paint left over will kinda gum up most flap wheels, especially the thicker under coat. A combination of angle grinder and needle scaler would be sweet. I would not use any grinding discs. The green finger wheels are pretty sweet too and probably safer but I'd probably go wire wheel still.
I've done a ton of this on my 80... a ton... I've probably committed any number or every number of safety violations while grinding but... especially for someone new and using a grinder under a vehicle in tight spaces (which is the hardest):
Be careful of the clothes you wear. If a grinder kicks back you don't want it wrapping up your sweatshirt hood strings. I'd probably get a faceshield and wear goggles or safety glasses under that. A half mask respirator would be ideal for this as well with the flat filters but at least use a cloth face mask. -- Nothing like black snot and hacking up crap. Gloves are always good. I have a bunch of scars from grinding discs and flap wheels... Wires fly everywhere so you're sure to get one stuck in your arm if you don't wear sleeves or in your eyes if you don't wear a face shield/glasses. OH and grinding discs and other crap, can and DO blow up. I've had a cut off wheel explode and a chunk puncture an aerosol can across the shop. Other people have had that s*** puncture their face. I've also heard of grinders kicking back and running up peoples clothes and getting wrapped up and against their face. Shoot the crap away from you and be careful how you use the grinder on angles or it will want to kick.
I've done a lot of grinding and very often not taken any safety precautions because I'm in a hurry and the worst that's happened is a few pieces of s*** in my eyes and some scars and that was lucky and stupid, it only takes once to lose an eye or two... I also know people who have gotten metal embedded in their eyes. It begins to rust and they have to "drill" it out.
Get a fan if you can to blow on you while you grind.
Also, grinding dics will chew up the surface, they dig in, hard to do any clean work with them.. Flap discs work best if you want to do some finer grinding, they CAN grind down thick stuff and leave a very nice finish, they're easy to work and it's hard to take off too much material unless you try -- they don't deal well with thick paint or other crap though. The finger wheels and wire wheels mostly don't remove metal and leave a nice finish.
FWIW I'd probably rather mechanically remove the rust than try chemical means if the rust is widespread and significant, myself...
ALSO, a drill or even a die grinder air tool, etc... are no comparison to an angle grinder.