What package is this you're talking about? I know Delta will do custom grinds on Toyota F engine cams that people have had good reviews of.
What has me curious is if oversized valves would be worth the work required to make them work in an F head. At the very least porting/polishing & port matching the head and having the stock valves 3-angled would help airflow through the head.
If I was to really go for extra power with a 3FE I would first do the old "hot rod" tricks that have been shown to make a difference at lower RPMs (4K and below). As said before, the 4 main bearings prevent safely reaching high RPMs with these engines.
Already working on a 3F carby head that will sit on a 2F block, paid for hi compression pistons, new valves, RV cam, ARP rod bolts, and better valve springs. i will also be balancing the motor. Already have headers and a tub-style intake (rest of the world spec). My overall plan is to be able to wind it out to 5000rpm safely while making more power across the band.
From everyone i spoke to, there really isn't much more gain from the larger valving, there is also the risk of taking away too much material and having a wasted head, my environment doesn't help either (Dubai deserts @100-110F in summer) but i've taken precautions for that (Alum rad and subaru electric fans on condenser with clutch driven) Now its a matter of putting it all together since as usual.....waiting on parts.